Efficient 2 S 3 positronium production by stimulated decay from the 3 P 3 level

We investigate experimentally the possibility of enhancing the production of 2S3 positronium atoms by driving the 1S3-3P3 and 3P3-2S3 transitions, overcoming the natural branching ratio limitation of spontaneous decay from 3P3 to 2S3. The decay of 3P3 positronium atoms toward the 2S3 level has been efficiently stimulated by a 1312.2 nm broadband IR laser pulse. The dependence of the stimulating transition efficiency on the intensity of the IR pulse has been measured to find the optimal enhancement conditions. A maximum relative increase of ×(3.1±1.0) in the 2S3 production efficiency, with respect to the case in which only spontaneous decay is present, was obtained.